In a groundbreaking advance poised to redefine the landscape of photonics and quantum technologies, a team of researchers has unveiled a novel method to harness spin-orbit coupling in van der Waals (vdW) materials to generate optical vortices with unprecedented control and efficiency. This development stands at the intersection of two revolutionary fields: the emerging class of two-dimensional materials bound by van der Waals forces and the intricate manipulation of light’s angular momentum. By exploiting the unique spin-orbit interactions intrinsic to these atomically thin crystals, the study unlocks new pathways for generating optical vortices—structured beams of light that carry orbital angular momentum (OAM)—ushering in exciting prospects for future optical communication, microscopy, and quantum information processing.
Optical vortices distinguish themselves from conventional light beams by their helical wavefronts and central phase singularities, conferring upon them a twisted corkscrew shape. Such beams carry orbital angular momentum, enabling them to encode information in their twist pattern distinct from the spin angular momentum linked to light’s polarization. Optical vortices have captivated scientific and technological communities due to their potential to multiplex data channels, improve resolution beyond classical limits, and manipulate microscopic particles. However, traditional methods to generate these beams rely on bulky components like spatial light modulators or spiral phase plates, often limiting integration and dynamical control in compact photonic devices.
Enter van der Waals materials—an emerging family of atomically thin layered crystals including graphene, transition metal dichalcogenides (TMDs), and beyond—renowned for their extraordinary electronic, optical, and mechanical properties. These materials’ structural anisotropy and reduced dimensionality give rise to pronounced spin-orbit coupling effects, whereby the intrinsic spin of electrons becomes tightly linked with their momentum. Capitalizing on these inherent microscopic interactions, the research team demonstrated that vdW materials can act as ultrathin optical elements capable of directly converting spin angular momentum into orbital angular momentum, effectively serving as novel generators of optical vortices.
At the heart of this breakthrough lies the manipulation of spin-orbit coupling within these two-dimensional crystals to mold light’s polarization and phase simultaneously. This interplay is fundamental because spin-orbit coupling facilitates coupling between the light’s intrinsic spin (polarization) and extrinsic orbital motion (vortex formation). By precisely designing vdW heterostructures and tailoring their interaction with incident light through tailored crystal orientation and stacking, the team harnessed spin-dependent phase shifts that shape the emergent optical field’s helical wavefront.
The researchers achieved this feat by employing advanced fabrication techniques to create vdW material layers stacked with angstrom-level precision, allowing for tunable spin-orbit interaction strengths. This enabled generating optical vortices with high purity and customizable topological charges—parameters that dictate the number of twists or ‘windings’ of the phase front around the beam axis. These topological charges are critical because they define the information-carrying capacity and interaction modes of the vortex beam. The ability to produce diverse vortex states with singular ultrathin components promises compact, scalable photonic devices for next-generation communications architecture.
One especially compelling aspect of the study is the dynamic tunability and integrability of these vdW-based vortex generators. Unlike static diffractive optics, vdW materials can respond to external stimuli such as electric fields, strain, or stacking sequences, providing actively reconfigurable control over the generated optical vortices. This versatility opens avenues for real-time modulation of vortex beams, a feature crucial for adaptive quantum networks and programmable photonic circuits. Moreover, the ultrathin nature of vdW materials eases on-chip integration with existing silicon photonics platforms, bridging a valuable gap between quantum photonics and mainstream photonic technology.
The implications of this discovery extend far beyond optical communications. The precise control of spin-orbit coupling in vdW materials ushers in new experimental regimes to explore light-matter interactions at the nano- and quantum scale. For instance, tailored optical vortices can interact uniquely with chiral molecules, enabling sensitive detection schemes for biomolecules or enantiomers. Additionally, the phenomenon holds promise for enhancing optical tweezers and nanoparticle manipulation, where the angular momentum of light exerts torque and forces at microscopic scales. By leveraging vdW spin-orbit effects, customized optical traps with enhanced functionality can be envisaged.
From a fundamental physics standpoint, the ability to convert spin angular momentum to orbital angular momentum in these versatile materials challenges and enriches our understanding of quantum electrodynamics in reduced dimensions. The fine interplay of spin, valley, and orbital degrees of freedom in two-dimensional crystals represents a fertile ground for discovering novel quantum phases and topological phenomena. The study’s approach accelerates such explorations by offering an experimental toolkit to probe spin-orbit coupling tailored to specific optical responses, potentially spurring innovations in spintronics and valleytronics.
Technologically, the advances reported could reshape the design principles of integrated photonics, allowing for the miniaturization and multifunctionalization of devices that handle structured light. Data centers and telecommunication hubs stand to benefit hugely as these vdW materials enable multiplexing schemes based on both polarization and phase degrees of freedom. These schemes dramatically increase data throughput while reducing energy consumption and device footprints. Furthermore, the precision afforded by vdW spin-orbit coupling mechanisms may enhance optical quantum computing protocols, where information is encoded in complex photon states.
The study also highlights the challenges overcome by the research team in controlling fabrication imperfections and environmental interactions, which could otherwise degrade spin-orbit effects and optical vortex quality. Meticulous characterization methods, including near-field microscopy and polarization-resolved measurements, underpinned the verification of vortex generation and topological charge assignments. This rigorous approach ensures reproducibility and offers a blueprint for translating laboratory results into commercially viable technologies.
Looking forward, the authors envision integrating these vdW optical vortex generators into multifunctional photonic circuits embedded with detectors, modulators, and nonlinear elements. Such integration promises holistic systems capable of producing, controlling, and routing structured light signals on a chip. The researchers also propose exploring heterostructures combining different vdW crystals to fine-tune spin-orbit interactions beyond current limits. The adaptation of this platform toward mid-infrared or terahertz frequencies is another tantalizing direction, potentially impacting imaging and sensing technologies in those spectral regions.
Crucially, this work sits within the broader context of nanoscale control over light-matter interaction—a field that has revolutionized nanophotonics and quantum optical technologies over the past decade. By stepping beyond passive interaction to active spin-orbit coupling exploitation in vdW materials, this research marks a paradigm shift in functional optical element design. The scientific community is now equipped with new levers to engineer the spatial, spectral, and polarization properties of light with atomic precision, overcoming fundamental limitations of classical photonics.
In summary, the reported synergy between spin-orbit coupling phenomena and vdW van der Waals materials to generate optical vortices embodies a groundbreaking stride in photonic science and technology. The sophistication, control, and tunability demonstrated in this work promise to accelerate applications spanning telecommunications, quantum computing, biosensing, and beyond. As the practical realization of these concepts advances, the fusion of two-dimensional quantum materials with complex light manipulation may herald a new epoch where tailored light-matter interactions become foundational building blocks of future information and sensing technologies.
Subject of Research: Spin-orbit coupling in van der Waals materials for the generation of optical vortex beams
Article Title: Spin-orbit coupling in van der Waals materials for optical vortex generation
Article References:
Jo, J., Byun, S., Bae, M. et al. Spin-orbit coupling in van der Waals materials for optical vortex generation. Light Sci Appl 14, 277 (2025). https://doi.org/10.1038/s41377-025-01926-7
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